Founded in 2011 as Estudiantes de Caroni Fútbol Club, the club first reached the Venezuelan Segunda División in 2013. In 2015, after a merger with Fundación Academia Deportiva Lala, the club changed name to Asociación Civil LALA Fútbol Club.
In December 2020, LALA was changing its name to Bolívar Sport Club,[2] but the name change did not materialize. Later on, Bolívar S.C. were founded as an independent institution from LALA.